Chinese Journal of Environmental Engineering•2026•DOI: 10.12030/j.cjee.202507110
Algal-derived taste and odor compounds (2-methylisoborneol, 2-MIB, and geosmin, GSM) in drinking water sources are poorly removed by conventional treatment. This study systematically evaluated the standalone and combined performance of ozone micro-nano bubbles (O3-MNBs) oxidation and powdered activated carbon (PAC) adsorption for removing 2-MIB, GSM, and algal cells from source water. Results showed that O3-MNBs pre-oxidation achieved >97.5% removal of odorants at 400 ng·L−1 and 67.2% algal cell removal within 30 min. When applied as a deep treatment stage, the degradation rate constant (k) was 10.1%–25.6% higher than in pre-oxidation due to lower background matrix interference. Both pre-oxidation and deep treatment reduced effluent concentrations of 2-MIB and GSM to below 10 ng·L−1, with oxidation kinetics fitting pseudo-first-order models (R²>0.95). PAC adsorption of both compounds followed pseudo-second-order kinetics (R²>0.99), with GSM equilibrium adsorption capacity approximately 20.0% higher than that of 2-MIB. In pure water, adsorption capacity increased by >10.0% compared to raw water. Based on kinetic models, a quantitative prediction method was established for O3-MNBs oxidation and PAC adsorption processes, aiming to achieve efficient odorant removal and cost optimization, providing theoretical support for advanced drinking water purification and smart water plant construction.
Chinese Journal of Environmental Engineering•2026•DOI: 10.12030/j.cjee.202510028
This study investigates the aging mechanism of polystyrene microplastics (PS MPs) induced by ultraviolet (UV)-activated potassium persulfate (KPS) and its influence on the adsorption of norfloxacin (NOR). Results show that aged PS exhibited yellowing, increased surface roughness and specific surface area, enhanced oxygen-containing functional groups, and elevated negative surface charge, along with the generation of environmentally persistent free radicals (EPFRs). Compared with UV alone, UV+KPS induced more pronounced aging due to the generation of reactive oxygen species (ROS) including hydroxyl radicals (·OH) and superoxide radicals (O2·−). Adsorption kinetics and isotherm data revealed that UV+KPS-aged PS significantly enhanced NOR adsorption, with a maximum adsorption capacity of (2.539±0.032) mg·g−1, which was 4.20 times higher than that of pristine PS. The adsorption mechanism was governed by hydrogen bonding, electrostatic interactions, and pore filling. Solution pH modulated the electrostatic interactions by affecting NOR speciation and PS surface charge, thereby influencing NOR adsorption. This study systematically reveals the accelerated aging of coexisting MPs and EPFRs generation during UV+KPS treatment, contributing to a comprehensive understanding of MPs environmental behavior and potential ecological risks.
Chinese Journal of Environmental Engineering•2026•DOI: 10.12030/j.cjee.202509067
Marine litter poses a significant threat to coastal ecosystems globally, necessitating a comprehensive understanding of its multi-compartment distribution and driving mechanisms for effective management. This study investigated the occurrence, composition, and sources of beach, sea surface, and seafloor litter in the northeastern Daya Bay, a semi-enclosed bay, during August–October 2024. Sampling included 11 beach transects, 6 surface transects, and 25 seafloor transects. Results showed that the mean density of large and very large beach litter was 4.41×10^5 items·km−2, while medium beach litter reached 5.39×10^6 items·km−2. Surface litter densities were 5.82×10^2 and 9.90×10^3 items·km−2 for large/very large and medium fractions, respectively. Seafloor litter averaged 5.20×10^3 items·km−2. Plastics dominated all compartments, accounting for 74.0% (beach), 96.0% (surface), and 78.8% (seafloor) of total litter. Source apportionment using NOWPAP methodology indicated that beach and surface litter primarily originated from coastal recreational activities, whereas seafloor litter was mainly derived from shipping and fishing. Beach quality assessment revealed that 63.6% of beaches were moderately clean or better (grade II–IV), and 90.9% were moderately safe or better (grade I–III). Hotspots included tourism beaches, tidal gyre areas, coral reef zones, and fishing grounds. The study underscores the need for targeted management, including improved waste collection on tourist beaches, dynamic cleaning protocols, and port reception facilities for fishing waste.
Environmental Chemistry•2026•DOI: 10.7524/j.issn.0254-6108.2025030501
Coastal areas serve as critical ecological interfaces for the migration of terrestrial microplastics (MPs) into the ocean, and characterizing their pollution is essential for integrated coastal management. This study investigated the occurrence, sources, and ecological risks of MPs in surface waters of nearshore areas and river estuaries around Hainan Island, a typical tropical tourist island. MPs abundance ranged from 316.67 to 1300 n·m−3 in seawater and from 400 to 5416.67 n·m−3 in river water. In seawater, the dominant polymer was polyethylene terephthalate, with fibers being the predominant shape, size class 500–1000 μm, and white/transparent color. In river water, polypropylene-ethylene copolymer dominated, also as fibers, but with size class 100–500 μm and white/transparent color. Seawater MP abundance showed a significant positive correlation with tourist numbers, and distribution across functional areas followed: tourism areas > natural areas > aquaculture areas > residential areas. Multiple correspondence analysis identified household plastic waste, laundry wastewater, aquaculture, and fishery products as primary sources of seawater MPs. Principal component analysis indicated homologous characteristics between seawater and river MPs, suggesting rivers are a major pathway for terrestrial MP transport to coastal zones. Ecological risk assessment revealed low pollution loads, with potential ecological risks moderate for seawater and medium-low for river water. Notably, 15% of seawater sampling sites exhibited polymer risk level Ⅳ, primarily driven by polyacrylonitrile's high biological toxicity. These findings provide a scientific basis for developing MP pollution control strategies in Hainan Island.
SCIENCE CHINA Materials•2026•DOI: 10.1007/s40843-025-3997-9
Contactless human-machine interaction (HMI) is rapidly evolving, yet it remains constrained by the latency, redundancy, and power consumption inherent in conventional frame-based vision sensors. While bio-inspired event-driven sensors offer a low-power alternative, existing architectures are often complex or fail to accurately encode the magnitude of light intensity changes. Herein, we report a solution-processed, two-terminal event-driven sensory device based on CuIn(Se,S)2 colloidal quantum dots (QDs) integrated with an Sb-doped TiO2 layer. Unlike traditional dynamic vision sensors (DVS), this device exhibits a transient photoresponse that encodes both the polarity and the magnitude of light intensity variations into the output current amplitude. This preservation of magnitude information significantly enhances the feature extraction capability, leading to faster convergence and superior clustering performance in gesture recognition. Based on these unique optoelectronic properties, we constructed a hierarchical HMI system that synergizes the strengths of event-based and frame-based sensing. The system utilizes the event-driven sensor for low-latency gesture control of an unmanned aerial vehicle (UAV) and a frame-based sensor for high-precision gaze control of an unmanned ground vehicle (UGV). The proposed system achieves a gesture recognition accuracy of more than 92.5% while substantially reducing data redundancy, offering a promising strategy for efficient, robust, and low-cost intelligent interaction systems.
SCIENCE CHINA Materials•2025•DOI: 10.1007/s40843-025-3435-3
Semiconductor nanowires (NWs) have been extensively applied in light sources, waveguides, and photodetectors (PDs), providing abundant components for optoelectronic interconnection applications. However, the efficient in-plane integration of various devices remains challenging, which is a prerequisite for the practical application of NWs. Here, the growth-based integration of CsPbBr3 NW arrays with CdSSe ribbons transferred onto mica is achieved via a vapor deposition route. The transferred ribbons not only act as preferential nucleation sites for CsPbBr3, but also break the growth symmetry of CsPbBr3 NWs on mica, allowing wires with the largest angle to the ribbon edge to grow longer and form arrays. The waveguide studies show that the CsPbBr3 NW arrays can confine and guide the light emission from both themselves and the CdSSe ribbon well. Importantly, the optoelectronic interconnection was successfully demonstrated based on the achieved heterostructures, where the CsPbBr3 NWs served as the light source and waveguide, and PDs were made from the CdSSe ribbon. When a single CsPbBr3 NW was illuminated by a focused 457 nm laser at a distance of 37.5 μm from the CdSSe ribbon, the on/off ratio of the system reached 8.3×10^3, resulting from the efficient response of the PD to the guided light. Moreover, the system can distinguish the pulsed light excitation well below 2000 Hz, limited by the response speed of the PDs. This work paves the way for the on-chip integration of nanoscale light emitters, waveguides, and detectors, promoting the practical application of semiconductor NWs in photonic circuits.