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JY
Verified CAS / Academic Author2 Decoded Studies

Prof. JIANG Yang

School of Metallurgy and Environment, Central South University, Changsha 410083, China

Research Publications & English Decoded Briefs

Showing 2 publications
Chinese Journal of Environmental Engineering2026DOI: 10.12030/j.cjee.202507058

Research Progress on Recycling Technologies for Cathode Materials of Spent Lithium Iron Phosphate Batteries

With the rapid development of China's lithium-ion power battery industry, the recycling of large-scale retired batteries has become a critical link for the sustainable development of the new energy vehicle industry. The recovery of cathode materials from spent lithium iron phosphate (LiFePO4) batteries is a current research hotspot, significant for resource recycling and environmental protection. This study systematically reviews recent progress in recycling technologies for spent LiFePO4 cathode materials, mainly including direct regeneration, pyrometallurgy, and hydrometallurgy. It focuses on analyzing the current research status of key steps in hydrometallurgy, such as leaching of valuable elements, deep removal of impurities, and product regeneration, and compares the advantages and limitations of various methods. Addressing core issues in current recovery processes, such as insufficient high-value utilization of iron and phosphorus resources and difficulty in deep impurity removal, this study proposes corresponding solutions and technical prospects, aiming to provide theoretical reference and engineering guidance for efficient, clean, and high-value recycling of spent LiFePO4 batteries.

SCIENCE CHINA Materials2026DOI: 10.1007/s40843-026-4147-9

Moisture-resistant and long-life fiber-shaped zinc-air batteries via electrolyte engineering

Fiber-shaped zinc-air batteries (FZABs) with aqueous electrolytes combine intrinsic safety, high energy density (1086 Wh kg−1), and environmental compatibility, making them attractive for wearable applications. However, free water in the electrolyte induces severe anode degradation while being a critical reactant for cathode redox, presenting a dilemma between anode stability and cathode functionality. The semi-open structure of FZABs allows airborne water to permeate and migrate to the anode, causing interfacial instability, while high surface area accelerates solvent evaporation, leading to increased internal resistance and salt crystallization. Consequently, typical cycle life is limited to <50 h. To overcome these challenges, we report a polymer electrolyte that captures atmospheric water as a solvent through the semi-open structure, achieved by introducing acetamide (AA), identified via unsupervised clustering algorithms, into the poly(vinylidene fluoride-hexafluoropropylene)/zinc trifluoromethanesulfonate (PVDF-HFP/Zn(OTf)2) system. AA incorporation preserves solvent-retention capability while reconstructing the Zn2+ coordination structure, promoting salt dissociation and polymer-segment mobility. Low adsorption energy of AA on zinc surfaces suppresses parasitic reactions from ambient moisture, and preferential adsorption across zinc crystal planes directs Zn2+ deposition along the (002) face, leading to uniform plating morphology. The exogenous aqueous polymer electrolyte exhibits superior mechanical properties, enabling stable output even after compression by a 1.7-t vehicle. As proof-of-concept, FZABs integrated with fiber solar cells and sensors in clothing enabled real-time health monitoring and sustainable energy utilization, demonstrating promising practical applications.