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Two-dimensionally confined Ir/WOx heterointerfaces boost the acidic oxygen evolution reaction for ampere-level stable PEM water electrolysis

Authors: Junlin Cai; Hongpu Huang; Weizhen Chen; Yuhang Peng; Luhong Fu; Shupeng Wang; Zhongyuan Zou; Zhichao Fu; Xiaohong Wang; Zhaoxiong Xie; Shuifen Xie

DOI: 10.1007/s40843-025-3398-9Status: Verified Translated Edition
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Key Findings in This Report

• • The Ir/WOx NSs achieve a mass activity of 2.34 A mgIr−1 at 300 mV overpotential, 11.1× and 9.8× higher than Ir NSs and commercial Ir/C, respectively, enabling significant reduction in Ir loading for cost-effective PEMWE deployment. • • The catalyst exhibits a low overpotential of 216 mV at 10 mA cm−2geo, surpassing commercial IrO2 and indicating enhanced intrinsic activity for acidic OER. • • In a PEM electrolyzer, Ir/WOx NSs deliver 1.0 A cm−2 at a cell voltage of 1.71 V, meeting ampere-level operational requirements for industrial hydrogen production. • • Long-term stability tests show a potential decay rate of only 2.8 μV h−1, compared to 210 μV h−1 for commercial IrO2, under dynamic current densities (0.2–1.0 A cm−2), demonstrating robust durability essential for intermittent renewable energy integration.