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Ultrafast dual-pathway room-temperature synthesis of 0D inorganic metal halides K3SbCl6 with near-unity photoluminescence quantum yield

Authors: YANG Maohao; GE Wanyin; ZHANG Qian; GUO Yao

DOI: 10.1007/s40843-025-4084-1Status: Verified Translated Edition
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Key Findings in This Report

• • Room-temperature grinding synthesis achieves structural evolution from KCl:Sb3+ to 0D K3SbCl6, yielding near-unity PLQY (approaching 100%), enabling high-efficiency solid-state lighting without high-temperature processing. • • Ultrafast single-crystal growth via solid-liquid interface diffusion completes in 20 seconds, drastically reducing production time compared to conventional slow evaporation or Bridgman methods, facilitating rapid manufacturing. • • Temperature sensing in 50–310 K range achieves maximum relative sensitivity of 9.99%/K, outperforming many existing optical thermometers, enabling precise cryogenic thermometry. • • Demonstrated multifunctionality in information encryption, flexible films, and white LEDs, with stable luminescence, indicating commercial viability for anti-counterfeiting and display technologies.