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Official PDF TranslationSCIENCE CHINA Materials

Towards Chlorine-Tolerant Seawater Electrolysis: Anode Electrocatalysts, Electrolyte, and System Design Strategies

Authors: Junnan Song; Xu Zhang; Guiqiang Pu; Zhenjie Cheng; Chenglong Qiu; Jiacheng Wang

DOI: 10.1007/s40843-025-3865-1Status: Verified Translated Edition
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Key Findings in This Report

• • Seawater contains ~0.5 M Cl− ions, which at high current densities can oxidize to chlorine or hypochlorite, competing with the oxygen evolution reaction (OER) and reducing Faraday efficiency while corroding the electrolytic cell. • • The review systematically categorizes chloride suppression strategies into three areas: directional catalyst design for OER, electrolyte composition optimization, and electrolytic cell engineering, each targeting the mitigation of chlorine-induced side reactions. • • Industrial-scale SWE requires addressing both efficiency and durability; the review emphasizes that without effective chloride suppression, the lifespan of electrolytic cells is curtailed, hindering commercialization. • • The review highlights that future development must focus on integrating these strategies to achieve stable, high-efficiency seawater electrolysis, with the goal of meeting projected hydrogen demand of at least 148 million tons annually by 2050.