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The interface interaction of sulfur-doped carbon boosting kinetics of Na4Fe3(PO4)2(P2O7) for high rate and stable sodium-ion batteries

Authors: CAI Yuyang; CHENG Hanwen; CHEN Zhuo; XU Hantao; LI Shidong; LI Jinghao; ZHANG Yibo; ZHAO Li; DOU Zhenzhen; XU Lin

DOI: 10.1007/s40843-025-3516-2Status: Verified Translated Edition
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Key Findings in This Report

• • NFPP-U0.5% delivers 80.3 mAh g−1 at 20 C, enabling high-power sodium-ion battery operation with minimal capacity fade under fast discharge conditions. • • Capacity retention of 82.66% after 25,000 cycles at 20 C demonstrates exceptional long-term cycling stability, surpassing typical polyanion cathodes and reducing replacement costs in grid-scale storage. • • The C–S–Fe interaction induces small lattice volume changes during cycling, as confirmed by in-situ XRD, mitigating mechanical degradation and extending electrode lifespan. • • S-doped carbon coating with porous coral-like morphology enhances electronic conductivity and Na+ diffusion, addressing the intrinsic limitations of NFPP and enabling practical high-rate performance.