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Stable-wavelength perovskite nanoplatelet laser via mixed-phase engineering

Authors: Guohui Li; Yulong Ji; Ruofan Zhao; Lin Xue; Ye Zhang; Kaibo Zheng; Yanxia Cui

DOI: 10.1007/s40843-025-3513-6Status: Verified Translated Edition
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Key Findings in This Report

• • At 163 K, mixed-phase MAPbI3 nanoplatelets achieve zero wavelength shift under pump density variation, eliminating a critical instability that plagues perovskite lasers for interferometric and quantum applications. • • Lasing threshold drops from 18.4 μJ cm⁻² at 293 K to 4.5 μJ cm⁻² at 163 K, a 75.5% reduction, enabling lower-power operation and reduced thermal load in integrated photonic circuits. • • Tetragonal phase exhibits a blueshift of 0.4 nm μJ⁻¹ cm², while orthorhombic phase shows a redshift of 1 nm μJ⁻¹ cm²; the opposing signs allow cancellation in the mixed phase, with a thermo-optic coefficient of 7.5 × 10⁻⁴ K⁻¹. • • Finite element simulations validate experimental shifts: tetragonal resonance moves from 780.86 nm at 296.62 K to 779.66 nm with a 10.70 K rise; orthorhombic shifts from 794.78 nm to 796.50 nm with a 1.69 μJ cm⁻² pump increase, confirming the mechanism for phase-dependent stability.