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Official PDF TranslationEnvironmental Chemistry

Research Progress on Potassium Permanganate Activated by Carbon Materials for Degradation of Organic Pollutants

Authors: LI Junjie; LIANG Zhijie; ZHANG Jing; MA Jun

DOI: 10.7524/j.issn.0254-6108.2024120203Status: Verified Translated Edition
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Key Findings in This Report

• • Carbon materials significantly enhance KMnO4 oxidation, with graphene oxide accelerating degradation of trace organic pollutants like sulfisoxazole, sulfamethazine, and bisphenol A, as demonstrated by Wang et al. • • Two primary mechanisms drive pollutant degradation in KMnO4/CMs systems: electron transfer mediation by carbon materials and generation of reactive manganese species, with carbon materials acting as electron transfer mediators to accelerate electron transfer between pollutants and KMnO4. • • Regeneration of deactivated carbon materials is achievable: thermal treatment at >350 °C under inert gas or chemical reduction removes surface oxygen groups, restoring catalytic performance; for example, reduced graphene oxide pyrolyzed at 700 °C for 2 h under nitrogen regained its sp2 structure and catalytic activity. • • Organic solvent washing (e.g., ethanol, hexane, acetone) or ultrasonic treatment can remove adsorbed intermediates or MnO2 deposits, recovering catalytic activity without structural damage, as shown for graphite.