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Microcrystallization-Gelation Enabled Mechanocompatible and Antibacterial Hydrogels for Cartilage Repair

Authors: Tailong Shi; Yan-Hua Xiong; Cheng Shen; Zongpeng Xiu; Lujiao Zhang; Ruonan Wu; Yang Li; Shun Duan; Tan Guo; Fu-Jian Xu

DOI: 10.1007/s40843-025-3646-1Status: Verified Translated Edition
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Key Findings in This Report

• • The optimal hydrogel formulation achieves a compressive modulus of 0.2 MPa and tensile strength of 2.2 MPa, matching human cartilage mechanical benchmarks, enabling load-bearing support in joint defects. • • The hydrogel withstands 50,000 compression cycles without structural failure, indicating fatigue resistance critical for long-term in vivo performance under cyclic joint loading. • • Incorporation of gentamicin confers antibacterial activity, addressing infection risks in cartilage repair, while nano-hydroxyapatite promotes osteogenesis for osteochondral integration. • • The material exhibits excellent flowability pre-crosslinking, allowing minimally invasive injection and adaptation to irregular defect geometries, a key advantage over pre-formed implants.