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Official PDF TranslationEnvironmental Chemistry

Excitation of Triplet State Dissolved Organic Matter Sensitizes Formic Acid to Generate CO2•− and Its Reductive Degradation of Metronidazole

Authors: WANG Jin; HOU Jie; LIU Huaying; ZHAO Qilin; SUN Donggou; LI Yingjie

DOI: 10.7524/j.issn.0254-6108.2024120701Status: Verified Translated Edition
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Key Findings in This Report

• • CO2•− generated via 3CBBP* oxidizing HCOO− achieved 98.2% degradation of 10 μmol·L−1 metronidazole within 30 min under 8 mmol·L−1 HCOO− and 200 μmol·L−1 CBBP, demonstrating a highly efficient reductive degradation route for recalcitrant pollutants. • • The degradation efficiency increased with HCOO− concentration (up to 8 mmol·L−1) and remained unaffected across pH variations, indicating robustness for applications in diverse water chemistries without pH adjustment. • • Common anions (Cl−, NO3−, CO3^2−, low HCO3−) inhibited MNZ degradation, whereas high HCO3− (≥? mmol·L−1) slightly enhanced it; humic acid (HA) suppressed degradation proportionally to its concentration, highlighting matrix-specific interference that must be managed in real water treatment. • • The hν/CBBP/HCOO− system exhibited effective MNZ degradation in real water samples, underscoring its practical viability for treating micropollutants in natural and engineered aquatic systems.