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Circularly Polarized Photoluminescence and Electroluminescence of a Pair of Eu(III) Enantiomers Based on Chiral Phosphine-Oxide Ligands

Authors: Si-Wei Wei; Zhong-Zhong Huo; Yi Wei; Yi-Fan Yang; Jia-Zhen Zhu; Jia-Qi Xi; Li Yuan; Chuanlang Zhan; You-Xuan Zheng

DOI: 10.1007/s40843-026-4105-8Status: Verified Translated Edition
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Key Findings in This Report

• • The R/S-Eu(TTA)3DFPO enantiomers exhibit a photoluminescence quantum yield of 43% and a narrowband red emission at 617 nm with a full width at half maximum of 11 nm, enabling high color purity for display applications. • • The |g_PL| value reaches 8.0 × 10^-3 at 590 nm (5D0→7F1 transition), demonstrating significant chiroptical activity in solution, which is essential for 3D display technologies. • • Vacuum-deposited CP-OLEDs achieve a maximum external quantum efficiency of 4.0% and |g_EL| values above 1.0 × 10^-2, indicating that the chiral Eu(III) complexes can be effectively integrated into device architectures without compromising efficiency. • • The use of point-chiral phosphine-oxide ancillary ligands ensures coordination stability, as evidenced by the successful fabrication of CP-OLEDs, addressing the bottleneck of maintaining chirality and stability in lanthanide complexes for practical applications.