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Official PDF TranslationJournal of Fuel Chemistry and Technology

Catalytic Conversion of Carbohydrates: Opportunities and Challenges en Route to Fuels and Chemicals

Authors: LUO Yang; LING Wenmeng; WANG Chenguang

DOI: 10.1016/S1872-5813(26)60651-2Status: Verified Translated Edition
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Key Findings in This Report

• • The review emphasizes catalytic conversion of carbohydrates using Brønsted and Lewis acids, targeting platform chemicals like 5-hydroxymethylfurfural (HMF), lactic acid, and furfural, with yields often exceeding 70% under optimized conditions, enabling cost-competitive bio-based production. • • Hydrolysis, isomerization, and dehydration are core reactions; for instance, glucose-to-fructose isomerization achieves equilibrium conversion of ~50% at 100°C with Lewis acid catalysts, a critical step for HMF synthesis. • • Subsequent derivatization of platform compounds yields bio-fuels and battery materials; for example, HMF derivatives like 2,5-dimethylfuran (DMF) have energy densities comparable to gasoline (33 MJ/L), making them viable fuel additives. • • The review identifies challenges in catalyst stability and selectivity, particularly in aqueous-phase reforming (APR) of polyols, where Pt-based catalysts show deactivation due to sintering, but bimetallic Pt-Re systems maintain >80% hydrogen selectivity over 100 hours on stream.