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Catalyst Enantiomer Purity Regulation Strategy for Accessing Chiral Poly(2-hydroxybutyric-co-glycolic acid) with Tunable Properties

Authors: Hassan Ahmed; Xuanhua Guo; Guangqiang Xu; Qinggang Wang

DOI: 10.1007/s40843-025-3718-3Status: Verified Translated Edition
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Key Findings in This Report

• • The catalyst enantiomer purity regulation strategy enables precise control over regioselectivity in ring-opening polymerization, yielding chiral poly(2-hydroxybutyric-co-glycolic acid) with G–G linkage contents varying from X% to Y% (exact values not provided in the text, but the strategy allows tunability). • • Thermo-mechanical properties, including glass transition temperature (Tg) and tensile modulus, are directly correlated with polymer microstructure; adjusting catalyst enantiomer purity allows modulation of Tg over a range of Z°C (exact values not specified). • • This approach circumvents the need for synthesizing multiple ligand variants, offering a more efficient route to tune polymer properties compared to traditional ligand regulation strategies. • • The synthesized chiral polymers exhibit tunable properties that are essential for biomedical applications, where degradation rates and mechanical performance must be matched to specific clinical requirements.