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Blended phase separation strategy for seamless integration of ultrathin crystalline channels and charge trapping layers toward multimode neuromorphic optoelectronics

Authors: WU Xianshuo; REN Yiwen; ZHANG Yihan; SUN Lingjie; WANG Zhaofeng; HU Suhao; XIE Yidi; DU Yuhan; LI Rongjin; ZHANG Xiaotao; YANG Fangxu

DOI: 10.1007/s40843-025-3593-5Status: Verified Translated Edition
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Key Findings in This Report

• • Photodetector performance: responsivity of 4.7 × 10^4 A/W, specific detectivity of 2.2 × 10^17 Jones, and photosensitivity of 1.5 × 10^8. These metrics exceed most organic photodetectors, enabling high-sensitivity image sensing for neuromorphic vision systems. • • Energy consumption per synaptic spike: 0.021 fJ for a single spike and 0.018 fJ average under two consecutive stimuli. These values are significantly lower than biological synaptic events (≈10 fJ) and most organic artificial synapses, critical for low-power neuromorphic computing. • • Flexible 7 × 7 synaptic array: under mechanical deformation, the array captured and retained a high-contrast 'T'-shaped image immediately after light exposure, with gradual decay emulating biological forgetting. This demonstrates viability for deformable, low-voltage neuromorphic systems. • • Dual-mode operation: gate-voltage-controlled switching between photo-switching (negative bias) and photonic synaptic (positive bias) modes within a single device. This enables logic gate functions (AND, OR) and synaptic plasticity (EPSC, PPF, STP-to-LTP) without additional components, reducing fabrication complexity.